It's from their 1992 album Iris, the cover art of which is a closeup of a human iris -- and also, I notice now, some "leaves of gold" imagery. There is no white of the eye, just a disembodied iris and pupil:
Today, clicking for a random /x/ thread en route to archive.org, I got one from 2014 called "eyes , post them." As might be expected, most of the posts are photos of eyes -- sometimes a single eye, sometimes a pair, but almost always a complete eye or eyes. The image in the original post, though, is a close-up of just the iris and pupil:
One of the images in this sync is a blue eye, and the other a reddish one, thus synching with the "Red and blue spectacles" theme. The names Joan and Iris have of course also been important in syncs, and the "milk-white steed" in the song may relate to the Four Horsemen syncs (e.g. "Flour Boy symbolism roundup").


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